Я могу использовать инициализатор набора для Словаря <TKey, TValue> записи?

Объединив динамическое решение Ege с идеей Vinay, вы получите хорошее надежное решение:

Array.prototype.sortBy = function() {
    function _sortByAttr(attr) {
        var sortOrder = 1;
        if (attr[0] == "-") {
            sortOrder = -1;
            attr = attr.substr(1);
        }
        return function(a, b) {
            var result = (a[attr] < b[attr]) ? -1 : (a[attr] > b[attr]) ? 1 : 0;
            return result * sortOrder;
        }
    }
    function _getSortFunc() {
        if (arguments.length == 0) {
            throw "Zero length arguments not allowed for Array.sortBy()";
        }
        var args = arguments;
        return function(a, b) {
            for (var result = 0, i = 0; result == 0 && i < args.length; i++) {
                result = _sortByAttr(args[i])(a, b);
            }
            return result;
        }
    }
    return this.sort(_getSortFunc.apply(null, arguments));
}

Использование:

// Utility for printing objects
Array.prototype.print = function(title) {
    console.log("************************************************************************");
    console.log("**** "+title);
    console.log("************************************************************************");
    for (var i = 0; i < this.length; i++) {
        console.log("Name: "+this[i].FirstName, this[i].LastName, "Age: "+this[i].Age);
    }
}

// Setup sample data
var arrObj = [
    {FirstName: "Zach", LastName: "Emergency", Age: 35},
    {FirstName: "Nancy", LastName: "Nurse", Age: 27},
    {FirstName: "Ethel", LastName: "Emergency", Age: 42},
    {FirstName: "Nina", LastName: "Nurse", Age: 48},
    {FirstName: "Anthony", LastName: "Emergency", Age: 44},
    {FirstName: "Nina", LastName: "Nurse", Age: 32},
    {FirstName: "Ed", LastName: "Emergency", Age: 28},
    {FirstName: "Peter", LastName: "Physician", Age: 58},
    {FirstName: "Al", LastName: "Emergency", Age: 51},
    {FirstName: "Ruth", LastName: "Registration", Age: 62},
    {FirstName: "Ed", LastName: "Emergency", Age: 38},
    {FirstName: "Tammy", LastName: "Triage", Age: 29},
    {FirstName: "Alan", LastName: "Emergency", Age: 60},
    {FirstName: "Nina", LastName: "Nurse", Age: 54}
];

//Unit Tests
arrObj.sortBy("LastName").print("LastName Ascending");
arrObj.sortBy("-LastName").print("LastName Descending");
arrObj.sortBy("LastName", "FirstName", "-Age").print("LastName Ascending, FirstName Ascending, Age Descending");
arrObj.sortBy("-FirstName", "Age").print("FirstName Descending, Age Ascending");
arrObj.sortBy("-Age").print("Age Descending");